Not really ambient music, but it is remarkable how music sounded back then in 1967. Have a listen. Quite intereseting. Though I know, there has been Stockhausen and other experimental stuff, but his kinda sounds like even a predecessor of the first Tangerine Dream albums.
http://www.youtube.com/watch?v=_l6MuQHvVBI&feature=related
Der Eber ebt den ganzen Tag,
so viel zu eben er vermag.
Sein ganzes Leben
verbringt er mit Eben.
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My favourite radio station for over ten years...